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Abstract:

Under controlled laboratory conditions, lasers represent a source of energy with well-defined parameters suitable for mimicking phenomena such as ablation, disintegration, and plasma formation processes that take place during the hypervelocity atmospheric entry of meteoroids. Furthermore, lasers have also been proposed for employment in future space exploration and planetary defense in a wide range of potential applications. This highlights the importance of an experimental investigation of lasers’ interaction with real samples of interplanetary matter: meteorite specimens. We summarize the results of numerous meteorite laser ablation experiments performed by several laser sources—a femtosecond Ti:Sapphire laser, the multislab ceramic Yb:YAG Bivoj laser, and the iodine laser known as PALS (Prague Asterix Laser System). The differences in the ablation spots’ morphology and their dependence on the laser parameters are examined via optical microscopy, scanning electron microscopy, and profilometry in the context of the meteorite properties and the physical characteristics of laser-induced plasma.

Abstract:

Volcanic eruptions eject large amounts of ash and trace gases such as sulfur dioxide (SO2) into the atmosphere. A significant difficulty in mitigating the impact of volcanic SO2 clouds on air traffic safety is that these gas emissions can be rapidly transported over long distances. The use of space-borne instruments enables the global monitoring of volcanic SO2 emissions in an economical and risk-free manner. Within the European Space Agency (ESA) Sentinel-5p+ Innovation project, the S5P SO2 layer height (S5P+I: SO2LH) activities led to the improvements of the retrieval algorithm and generation of the corresponding near real-time S5P SO2 LH products. These are currently operationally provided, in near real-time, by the German Aerospace Center (DLR) within the framework of the Innovative Products for Analyses of Atmospheric Composition (INPULS) project. The main aim of this paper is to present its extensive verification, accomplished within the S5P+I: SO2LH project, over major recent volcanic eruptions, against collocated space-borne measurements from the IASI/Metop and CALIOP/CALIPSO instruments as well as assess its impact on the forecasts provided by the Copernicus Atmospheric Monitoring Service (CAMS). The mean difference between S5P and IASI observations for the Raikoke 2019, the Nishinoshima 2020 and the La Soufrière-St Vincent 2021 eruptive periods is ∼ 0.5 ± 3 km, while for the Taal 2020 eruption, a larger difference was found, between 3 ± 3 km and 4 ± 3 km. The comparison of the daily mean SO2 LH further demonstrates the capabilities of this near real-time product, with slopes between 0.8 and 1 and correlation coefficients ranging between 0.6 and 0.8. Comparisons between the S5P SO2 LH and the CALIOP/CALIPSO ash plumes revealed an expected bias at −2.5 ± 2 km, considering that the injected SO2 and ash plume locations do not always coincide over an eruption. Furthermore, the CAMS assimilation of the S5P SO2 LH product led to much improved model output against the non-assimilated IASI LH, with a mean difference of 1.5 ± 2 km, compared to the original CAMS analysis, and improved the geographical spread of the Raikoke volcanic plume following the eruptive days.

Abstract:

Volcanic eruptions eject large amounts of ash and trace gases such as sulfur dioxide (SO2) into the atmosphere. A significant difficulty in mitigating the impact of volcanic SO2 clouds on air traffic safety is that these gas emissions can be rapidly transported over long distances. The use of space-borne instruments enables the global monitoring of volcanic SO2 emissions in an economical and risk-free manner. Within the European Space Agency (ESA) Sentinel-5p+ Innovation project, the S5P SO2 layer height (S5P+I: SO2LH) activities led to the improvements of the retrieval algorithm and generation of the corresponding near real-time S5P SO2 LH products. These are currently operationally provided, in near real-time, by the German Aerospace Center (DLR) within the framework of the Innovative Products for Analyses of Atmospheric Composition (INPULS) project. The main aim of this paper is to present its extensive verification, accomplished within the S5P+I: SO2LH project, over major recent volcanic eruptions, against collocated space-borne measurements from the IASI/Metop and CALIOP/CALIPSO instruments as well as assess its impact on the forecasts provided by the Copernicus Atmospheric Monitoring Service (CAMS). The mean difference between S5P and IASI observations for the Raikoke 2019, the Nishinoshima 2020 and the La Soufrière-St Vincent 2021 eruptive periods is g-1/4 0.5 ± 3 km, while for the Taal 2020 eruption, a larger difference was found, between 3 ± 3 km and 4 ± 3 km. The comparison of the daily mean SO2 LH further demonstrates the capabilities of this near real-time product, with slopes between 0.8 and 1 and correlation coefficients ranging between 0.6 and 0.8. Comparisons between the S5P SO2 LH and the CALIOP/CALIPSO ash plumes revealed an expected bias at -2.5 ± 2 km, considering that the injected SO2 and ash plume locations do not always coincide over an eruption. Furthermore, the CAMS assimilation of the S5P SO2 LH product led to much improved model output against the non-assimilated IASI LH, with a mean difference of 1.5 ± 2 km, compared to the original CAMS analysis, and improved the geographical spread of the Raikoke volcanic plume following the eruptive days.

Abstract:

We have implemented a new stratospheric ozone model in the European Centre for Medium-Range Weather Forecasts (ECMWF) system and tested its performance for different timescales to assess the impact of stratospheric ozone on meteorological fields. We have used the new ozone model to provide prognostic ozone in medium-range and long-range (seasonal) experiments, showing the feasibility of this ozone scheme for a seamless numerical weather prediction (NWP) modelling approach. We find that the stratospheric ozone distribution provided by the new scheme in ECMWF forecast experiments is in very good agreement with observations, even for unusual meteorological conditions such as Arctic stratospheric sudden warmings (SSWs) and Antarctic polar vortex events like the vortex split of year 2002. To assess the impact it has on meteorological variables, we have performed experiments in which the prognostic ozone is interactive with radiation. The new scheme provides a realistic ozone field able to improve the description of the stratosphere in the ECMWF system, as we find clear reductions of biases in the stratospheric forecast temperature. The seasonality of the Southern Hemisphere polar vortex is also significantly improved when using the new ozone model. In medium-range simulations we also find improvements in high-latitude tropospheric winds during the SSW event considered in this study. In long-range simulations, the use of the new ozone model leads to an increase in the correlation of the winter North Atlantic Oscillation (NAO) index with respect to ERA-Interim and an increase in the signal-to-noise ratio over the North Atlantic sector. In our study we show that by improving the description of the stratospheric ozone in the ECMWF system, the stratosphere–troposphere coupling improves. This highlights the potential benefits of this new ozone model to exploit stratospheric sources of predictability and improve weather predictions over Europe on a range of timescales.