Magnetic excitations of the charge stripe electrons below half doping in La2-xSrxNiO4 (x = 0.45, 0.4)

Physical Review B American Physical Society 95:6 (2017) 064403

Authors:

PG Freeman, K Hradil, RA Mole, P Cermak, Dharmalingam Prabhakaran

Abstract:

The low energy magnetic excitation spectrum of charge stripe ordered La2-xSrxNiO4, x=0.4 and x=0.45 samples, were studied by neutron scattering. Two excitation modes are observed in both materials, one from the ordered magnetic moments, and a second mode consistent with pseudo-one-dimensional antiferromagnetic excitations of the charge stripe electrons (q-1D). The dispersion of the q-1D excitation follows the same relation as in x=1/3 composition, with even spectral weight in the two counterpropagating branches of the x=0.4 sample, however in the x=0.45 sample only one dispersion branch has any measurable spectral weight. The evolution of the q-1D excitations on doping to the checkerboard charge ordered phase is discussed.

Effect of doping and defects in pyrochlore compounds

ACTA CRYSTALLOGRAPHICA A-FOUNDATION AND ADVANCES 73 (2017) C1020-C1020

Authors:

Dharmalingam Prabhakaran, Sichen Wang, Richard Brearton, Andrew Boothroyd

Hall effect in charged conducting ferroelectric domain walls

Nature Communications Springer Nature 7:1 (2016) 13764

Authors:

MP Campbell, JPV McConville, RGP McQuaid, D Prabhakaran, A Kumar, JM Gregg

Layer-by-layer epitaxial thin films of the pyrochlore Tb2Ti2O7.

Nanotechnology Institute of Physics 28:5 (2016) 055708

Authors:

L Bovo, CM Rouleau, Dharmalingam Prabhakaran, ST Bramwell

Abstract:

Layer-by-layer epitaxial growth of the pyrochlore magnet Tb2Ti2O7 on the isostructural substrate Y2Ti2O7 results in high-quality single crystal films of up to 60 nm thickness. Substrate-induced strain is shown to act as a strong and controlled perturbation to the exotic magnetism of Tb2Ti2O7, opening up the general prospect of strain-engineering the diverse magnetic and electrical properties of pyrochlore oxides.

Crystal growth of the triangular-lattice antiferromagnet Ba3CoSb2O9

Journal of Crystal Growth Elsevier 468 (2016) 345-348

Authors:

Dharmalingam Prabhakaran, Andrew T Boothroyd

Abstract:

We report growth of large single crystals of the triangular-lattice antiferromagnetic compound Ba3CoSb2O9 by the floating-zone technique in an image furnace. Evaporation of Sb due to its high volatility was controlled by high pressure and addition of excess Sb in the starting materials to compensate for the losses. The crystal quality was analysed using different X-ray techniques, and the magnetic transition temperature was confirmed by magnetization and heat capacity measurements.