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Abstract:

Generalized string-net models have been proposed recently in order to enlarge the set of possible topological quantum phases emerging from the original string-net construction. In the present work we do not consider vertex excitations, and we restrict ourselves to plaquette excitations, or fluxons, that satisfy important identities. We explain how to compute the energy-level degeneracies of the generalized string-net Hamiltonian associated with an arbitrary unitary fusion category. In contrast to the degeneracy of the ground state, which is purely topological, the degeneracy of excited energy levels depends not only on the Drinfeld center of the category, but also on internal multiplicities obtained from the tube algebra defined from the category. For a noncommutative category, these internal multiplicities result in extra nontopological degeneracies. Our results are valid for any trivalent graph and any orientable surface. We illustrate our findings with nontrivial examples.

Abstract:

The dipolar-octupolar (DO) pyrochlores, R2M2O7 (R=Ce,Sm,Nd), are key players in the search for realizable novel quantum spin liquid (QSL) states as a large parameter space within the DO pyrochlore phase diagram is theorized to host QSL states of both dipolar and octupolar nature. New single crystals and powders of Ce2Sn2O7, synthesized by hydrothermal techniques, present an opportunity for a new characterization of the exchange parameters in Ce2Sn2O7 using the near-neighbor XYZ model Hamiltonian associated with DO pyrochlores. Utilizing quantum numerical linked cluster expansion fits to heat capacity and magnetic susceptibility measurements, and classical Monte Carlo calculations to the diffuse neutron diffraction of the new hydrothermally grown Ce2Sn2O7 samples, we place Ce2Sn2O7's ground state within the ordered dipolar all-in-all-out (AIAO) Néel phase, with quantum Monte Carlo calculations showing a transition to long-range order at temperatures below those accessed experimentally. Indeed, our new neutron diffraction measurements on the hydrothermally grown Ce2Sn2O7 powders show a broad signal at low scattering wave vectors, reminiscent of a dipolar spin ice, in striking contrast from previous powder neutron diffraction on samples grown from solid-state synthesis, which found diffuse scattering at high scattering wave vectors associated with magnetic octupoles and suggested an octupolar quantum spin ice state. We conclude that new hydrothermally grown Ce2Sn2O7 samples host a finite-temperature proximate dipolar spin ice phase, above the expected transition to AIAO Néel order.