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Abstract:

Aerosol effects on cloud properties and the atmospheric energy and radiation budgets are studied through ensemble simulations over two month-long periods during the NARVAL campaigns (Next-generation Aircraft Remote-Sensing for Validation Studies, December 2013 and August 2016). For each day, two simulations are conducted with low and high cloud droplet number concentrations (CDNCs), representing low and high aerosol concentrations, respectively. This large data set, which is based on a large spread of co-varying realistic initial conditions, enables robust identification of the effect of CDNC changes on cloud properties. We show that increases in CDNC drive a reduction in the top-of-atmosphere (TOA) net shortwave flux (more reflection) and a decrease in the lower-tropospheric stability for all cases examined, while the TOA longwave flux and the liquid and ice water path changes are generally positive. However, changes in cloud fraction or precipitation, that could appear significant for a given day, are not as robustly affected, and, at least for the summer month, are not statistically distinguishable from zero. These results highlight the need for using a large sample of initial conditions for cloud–aerosol studies for identifying the significance of the response. In addition, we demonstrate the dependence of the aerosol effects on the season, as it is shown that the TOA net radiative effect is doubled during the winter month as compared to the summer month. By separating the simulations into different dominant cloud regimes, we show that the difference between the different months emerges due to the compensation of the longwave effect induced by an increase in ice content as compared to the shortwave effect of the liquid clouds. The CDNC effect on the longwave flux is stronger in the summer as the clouds are deeper and the atmosphere is more unstable.

Abstract:

<jats:p>Abstract. Aerosol effects on cloud properties and the atmospheric energy and radiation budgets are studied through ensemble simulations over two month-long periods during the NARVAL campaigns (December 2013 and August 2016). For each day, two simulations are conducted with low and high cloud droplet number concentrations (CDNC), representing low and high aerosol concentrations, respectively. This large data-set, which is based on a large spread of co-varying realistic initial conditions, enables robust identification of the effect of CDNC changes on cloud properties. We show that increases in CDNC drive a reduction in the top of atmosphere (TOA) net shortwave flux (more reflection) and a decrease in the lower tropospheric stability for all cases examined, while the TOA longwave flux and the liquid and ice water path changes are generally positive. However, changes in cloud fraction or precipitation, that could appear significant for a given day, are not as robustly affected, and, at least for the summer month, are not statistically distinguishable from zero. These results highlight the need for using large statistics of initial conditions for cloud–aerosol studies for identifying the significance of the response. In addition, we demonstrate the dependence of the aerosol effects on the season, as it is shown that the TOA net radiative effect is doubled during the winter month as compared to the summer month. By separating the simulations into different dominant cloud regimes, we show that the difference between the different months emerge due to the compensation of the longwave effect induced by an increase in ice content as compared to the shortwave effect of the liquid clouds. The CDNC effect on the longwave is stronger in the summer as the clouds are deeper and the atmosphere is more unstable. </jats:p>

Abstract:

The uncertainty in present-day anthropogenic forcing is dominated by uncertainty in the strength of the contribution from aerosol. Much of the uncertainty in the direct aerosol forcing can be attributed to uncertainty in the anthropogenic fraction of aerosol in the present-day atmosphere, due to a lack of historical observations. Here we present a robust relationship between total present-day aerosol optical depth and the anthropogenic contribution across three multi-model ensembles and a large single-model perturbed parameter ensemble. Using observations of aerosol optical depth, we determine a reduced likely range of the anthropogenic component and hence a reduced uncertainty in the direct forcing of aerosol.