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Abstract:

There are two main theoretical descriptions of antiferromagnets. The first arises from atomic physics, which predicts that atoms with unpaired electrons develop magnetic moments. In a solid, the coupling between moments on nearby ions then yields antiferromagnetic order at low temperatures. The second description, based on the physics of electron fluids or 'Fermi liquids' states that Coulomb interactions can drive the fluid to adopt a more stable configuration by developing a spin density wave. It is at present unknown which view is appropriate at a 'quantum critical point' where the antiferromagnetic transition temperature vanishes. Here we report neutron scattering and bulk magnetometry measurements of the metal CeCu(6-x)Au(x), which allow us to discriminate between the two models. We find evidence for an atomically local contribution to the magnetic correlations which develops at the critical gold concentration (x(c) = 0.1), corresponding to a magnetic ordering temperature of zero. This contribution implies that a Fermi-liquid-destroying spin-localizing transition, unanticipated from the spin density wave description, coincides with the antiferromagnetic quantum critical point.

Abstract:

The spin excitations in La2CuO4, a two-dimensional spin- 1/2 Heisenberg antiferromagnet and parent compound of high-Tc superconductors, have been measured throughout the Brillouin zone using high-resolution inelastic neutron scattering. The observed dispersion relations show evidence for substantial second- or third-nearest-neighbour exchange couplings in addition to the strong first nearest-neighbour antiferromagnetic exchange.

Abstract:

Measurements of the magnetic-field dependent millimetre-wave response of Cs2CuCl4, a quasi-one-dimensional Heisenberg antiferromagnet, are presented. The evolution of the electron spin resonance between high temperatures (the paramagnetic regime) and temperatures below T-N, at which there is an onset of long-range magnetic order (the antiferromagnetic regime), is studied for a range of crystal orientations. The magneto-optical data suggest that there is an onset of local magnetic order at temperatures considerably higher than T-N as determined from neutron scattering measurements, and that the evolution towards a long-range ordered state is gradual. A phenomenological model that describes the general features is suggested. (C) 1998 Elsevier Science B.V. All rights reserved.