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Abstract:

Light fields at terahertz and mid-infrared frequencies allow for the direct excitation of collective modes in condensed matter, which can be driven to large amplitudes. For example, excitation of the crystal lattice has been shown to stimulate insulator-metal transitions, melt magnetic order or enhance superconductivity. Here, we generalize these ideas and explore the simultaneous excitation of more than one lattice mode, which are driven with controlled relative phases. This nonlinear mode mixing drives rotations as well as displacements of the crystal-field atoms, mimicking the application of a magnetic field and resulting in the excitation of spin precession in the rare-earth orthoferrite ErFeO 3. Coherent control of lattice rotations may become applicable to other interesting problems in materials research-for example, as a way to affect the topology of electronic phases.

Abstract:

Resonant excitation of local molecular vibrations at mid-infrared wavelengths is shown to induce a transient superconducting state in the organic superconductor K3C60 for temperatures far above the equilibrium critical temperature.